固态里德堡激子研究进展
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1.华中科技大学 光学与电子信息学院,湖北 武汉 430074
2.华中科技大学 武汉光电国家实验室,湖北 武汉 430074
3.山西大学 激光光谱研究所 光量子技术与器件全国重点实验室,山西 太原 030006

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Recent advances in solid-state Rydberg excitons
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1.School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, China
2.Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, China
3.State Key Laboratory of Quantum Optics Technologies and Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan 030006, China

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    摘要:

    介绍了里德堡激子作为半导体中高激发态电子空穴对的核心特征,包括类氢能级、宏观量子特性、强相互作用与非线性响应。阐述了氧化亚铜(Cu2O)因其低缺陷和偶极跃迁禁止特性,成为研究高阶里德堡态的理想平台。分析了利用光谱技术和外场调控揭示的里德堡激子特性——微米级半径、高极化率、长寿命和大偶极矩。探讨了高主量子数下激子间显著增强的长程相互作用及其引发的激子阻塞和非线性折射现象,以及外场对能级分裂、跃迁选择定则和选择性激发的调控作用,并提及环境扰动的影响。指出里德堡激子凭借其独特的物理性质和对环境的高度敏感性,在弱场传感、片上单光子器件、量子模拟及微波光学转换等前沿领域具有巨大应用潜力;深入研究和开发这些特性是未来实现高性能量子信息技术与精密传感技术的关键方向。

    Abstract:

    This review introduces Rydberg excitons as highly excited electron-hole pairs in semiconductors, highlighting their core characteristics: hydrogen-like energy levels, macroscopic quantum properties, strong interactions, and nonlinear optical response. It elaborates on cuprous oxide (Cu2O) as an ideal platform for observing high-order Rydberg states due to its low defect density and dipole-forbidden transitions. The analysis covers key properties of Rydberg excitons revealed through spectroscopic techniques and external field manipulation: micron-scale radii, high polarizability, long lifetimes, and large dipole moments. It further discusses the significantly enhanced long-range interactions between excitons at high principal quantum numbers, which lead to phenomena like excitonic blockade and nonlinear refraction. The discussion extends to the modulation of excitonic properties by external fields, including field-induced energy level splitting, alteration of transition selection rules, and selective excitation of specific states, while also noting the impact of environmental perturbations on spectral features. It is pointed out that Rydberg excitons have great potential for applications in cutting-edge fields such as weak-field sensing, on-chip single-photon devices, quantum simulation, and microwave-to-optical signal conversion due to their distinctive physical attributes and extreme sensitivity to external fields and the environment. The review proposes that in-depth research and exploitation of these properties represent a crucial direction for advancing high-performance quantum information technologies and precision sensing in the future.

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翟宇飞, 杨吕鹏, 邵明, 余宇, 汪毅, 张好, 马一飞, 王梅, 张临杰.固态里德堡激子研究进展[J].计测技术,2025,45(4):12~47:
10.11823/j. issn.1674-5795.2025.04.02.

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  • 在线发布日期: 2025-09-10
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